Recycling spent lithium-ion batteries (LIBs) has attracted lots of attention recently, due to the increasing demand for critical materials contained in LIBs, putting high pressure on their geological reserves. We evaluated the potential of bioleaching technology as a sustainable solution for recycling spent LIBs to help inform decision-making processes for stakeholders involved in LIB recycling supply chains. A supply chain model was developed to include required upstream processes with the objective of maximizing economic feasibility of LIB recycling through the technology. The model has been applied to the U.S. and an optimal supply chain configuration was identified, considering the major factors affecting the economic viability of the technology. The net present value of the supply chain was estimated to be $18.4 billion for operating over 10 years, achieving the maximum processing capacity of 900,000 tons of black mass per year. The economic viability of the technology was identified to be highly sensitive to the cost associated with purchasing black mass, which accounted for more than 60% of the total supply chain cost. The breakeven price of black mass was identified as $8.7/kg over which the supply chain was not economically sustainable. Additionally, we examined the non-cooperative scenarios where each tier tries to maximize its own profit to demonstrate how the overall profitability of the supply chain changes with different pricing strategies of sortation facilities and acid producers. We estimated that the maximum prices of non-recyclable paper and acid that the supply chain could tolerate were $0.89/kg and $8.5/kg, respectively, beyond which the supply chain was no longer sustainable.
Citation: Majid Alipanah, Sunday Oluwadamilola Usman, Apurba Kumar Saha, Hongyue Jin. Designing profitable supply chains for lithium-ion battery recycling in the United States[J]. Clean Technologies and Recycling, 2024, 4(1): 22-42. doi: 10.3934/ctr.2024002
Recycling spent lithium-ion batteries (LIBs) has attracted lots of attention recently, due to the increasing demand for critical materials contained in LIBs, putting high pressure on their geological reserves. We evaluated the potential of bioleaching technology as a sustainable solution for recycling spent LIBs to help inform decision-making processes for stakeholders involved in LIB recycling supply chains. A supply chain model was developed to include required upstream processes with the objective of maximizing economic feasibility of LIB recycling through the technology. The model has been applied to the U.S. and an optimal supply chain configuration was identified, considering the major factors affecting the economic viability of the technology. The net present value of the supply chain was estimated to be $18.4 billion for operating over 10 years, achieving the maximum processing capacity of 900,000 tons of black mass per year. The economic viability of the technology was identified to be highly sensitive to the cost associated with purchasing black mass, which accounted for more than 60% of the total supply chain cost. The breakeven price of black mass was identified as $8.7/kg over which the supply chain was not economically sustainable. Additionally, we examined the non-cooperative scenarios where each tier tries to maximize its own profit to demonstrate how the overall profitability of the supply chain changes with different pricing strategies of sortation facilities and acid producers. We estimated that the maximum prices of non-recyclable paper and acid that the supply chain could tolerate were $0.89/kg and $8.5/kg, respectively, beyond which the supply chain was no longer sustainable.
[1] | Li-cycle (2021) LI-CYCLE UPSIZED HUB AND STRATEGIC COLLABORATION WITH LG. Available from: https://li-cycle.com/in-the-news/li-cycle-to-expand-us-battery-recycling-hub-by-40-and-provide-lg-with-nickel-for-the-next-decade/ (last accessed on June 17, 2024) |
[2] | Alipanah M, Saha AK, Vahidi E, et al. (2021) Value recovery from spent lithium-ion batteries: A review on technologies, environmental impacts, economics, and supply chain. Clean Technol Recyc 1: 152–184. https://doi.org/10.3934/ctr.2021008 doi: 10.3934/ctr.2021008 |
[3] | Latini D, Vaccari M, Lagnoni M, et al. (2022) A comprehensive review and classification of unit operations with assessment of outputs quality in lithium-ion battery recycling. J Power Sources 546: 231979. https://doi.org/10.1016/j.jpowsour.2022.231979 doi: 10.1016/j.jpowsour.2022.231979 |
[4] | Jin S, Mu D, Lu Z, et al. (2022) A comprehensive review on the recycling of spent lithium-ion batteries: Urgent status and technology advances. J Clean Prod 340: 130535. https://doi.org/10.1016/j.jclepro.2022.130535 doi: 10.1016/j.jclepro.2022.130535 |
[5] | Gaines L (2018) Lithium-ion battery recycling processes: Research towards a sustainable course. Sustain Mater Techno 17: e00068. https://doi.org/10.1016/j.susmat.2018.e00068 doi: 10.1016/j.susmat.2018.e00068 |
[6] | Moazzam P, Boroumand Y, Rabiei P, et al. (2021) Lithium bioleaching: An emerging approach for the recovery of Li from spent lithium ion batteries. Chemosphere 277: 130196. https://doi.org/10.1016/j.chemosphere.2021.130196 doi: 10.1016/j.chemosphere.2021.130196 |
[7] | Huang B, Pan Z, Su X, et al. (2018) Recycling of lithium-ion batteries: Recent advances and perspectives. J Power Sources 399: 274–286. https://doi.org/10.1016/j.jpowsour.2018.07.116 doi: 10.1016/j.jpowsour.2018.07.116 |
[8] | Balchandani S, Alipanah M, Barboza CA, et al. (2023) Techno-economic analysis and life cycle assessment of gluconic acid and xylonic acid production from waste materials. ACS Sustainable Chem Eng 11: 17708–17717. https://doi.org/10.1021/acssuschemeng.3c05117 doi: 10.1021/acssuschemeng.3c05117 |
[9] | Toba AL, Nguyen RT, Cole C, et al. (2021) U.S. lithium resources from geothermal and extraction feasibility. Resour Conserv Recyc 169: 105514. https://doi.org/10.1016/j.resconrec.2021.105514 doi: 10.1016/j.resconrec.2021.105514 |
[10] | Wang L, Wang X, Yang W (2020) Optimal design of electric vehicle battery recycling network—From the perspective of electric vehicle manufacturers. Appl Energ 275: 115328. https://doi.org/10.1016/j.apenergy.2020.115328 doi: 10.1016/j.apenergy.2020.115328 |
[11] | Hoyer C, Kieckhä fer K, Spengler TS (2015) Technology and capacity planning for the recycling of lithium-ion electric vehicle batteries in Germany. J Bus Econ 85: 505–544. https://doi.org/10.1007/s11573-014-0744-2 doi: 10.1007/s11573-014-0744-2 |
[12] | Tadaros M, Migdalas A, Samuelsson B, et al. (2022) Location of facilities and network design for reverse logistics of lithium-ion batteries in Sweden. Oper Res-Ger 22: 895–915. https://doi.org/10.1007/s12351-020-00586-2 doi: 10.1007/s12351-020-00586-2 |
[13] | Hendrickson TP, Kavvada O, Shah N, et al. (2015) Life-cycle implications and supply chain logistics of electric vehicle battery recycling in California. Environ Res Lett 10: 014011. https://doi.org/10.1088/1748-9326/10/1/014011 doi: 10.1088/1748-9326/10/1/014011 |
[14] | Gonzales-Calienes G, Yu B, Bensebaa F (2022) Development of a reverse logistics modeling for end-of-life lithium-ion batteries and its impact on recycling viability—A case study to support end-of-life electric vehicle battery strategy in Canada. Sustainability 14: 15321. https://doi.org/10.3390/su142215321 doi: 10.3390/su142215321 |
[15] | Rosenberg S, Glö ser-Chahoud S, Huster S, et al. (2023) A dynamic network design model with capacity expansions for EoL traction battery recycling—A case study of an OEM in Germany. Waste Manage 160: 12–22. https://doi.org/10.1016/j.wasman.2023.01.029 doi: 10.1016/j.wasman.2023.01.029 |
[16] | Yükseltürk A, Wewer A, Bilge P, et al. (2021) Recollection center location for end-of-life electric vehicle batteries using fleet size forecast: Scenario analysis for Germany, Procedia CIRP 96: 260–265. https://doi.org/10.1016/j.procir.2021.01.084 doi: 10.1016/j.procir.2021.01.084 |
[17] | Zhang M, Wu W, Song Y (2023) Study on the impact of government policies on power battery recycling under different recycling models. J Clean Prod 413: 137492. https://doi.org/10.1016/j.jclepro.2023.137492 doi: 10.1016/j.jclepro.2023.137492 |
[18] | Zhao X, Peng B, Zheng C, et al. (2022) Closed-loop supply chain pricing strategy for electric vehicle batteries recycling in China. Environ Dev Sustain 24: 7725–7752. https://doi.org/10.1007/s10668-021-01755-9 doi: 10.1007/s10668-021-01755-9 |
[19] | Lin Y, Yu Z, Wang Y, et al. (2023) Performance evaluation of regulatory schemes for retired electric vehicle battery recycling within dual-recycle channels. J Environ Manage 332: 117354. https://doi.org/10.1016/j.jenvman.2023.117354 doi: 10.1016/j.jenvman.2023.117354 |
[20] | Gu SQ, Liu Y, Yu H (2023) Power battery recycling strategy with government rewards and punishments. Opsearch 60: 501–526. https://doi.org/10.1007/s12597-022-00618-9 doi: 10.1007/s12597-022-00618-9 |
[21] | Li X, Du J, Liu P, et al. (2023) Optimal choice of power battery joint recycling strategy for electric vehicle manufacturers under a deposit-refund system. Int J Prod Res 61: 7281–7301. https://doi.org/10.1080/00207543.2022.2148009 doi: 10.1080/00207543.2022.2148009 |
[22] | Alipanah M, Reed D, Thompson V, et al. (2023) Sustainable bioleaching of lithium-ion batteries for critical materials recovery. J Clean Prod 382: 135274. https://doi.org/10.1016/j.jclepro.2022.135274 doi: 10.1016/j.jclepro.2022.135274 |
[23] | AMP Robotics (2023). Available from: https://amp-robotics.squarespace.com/about-us. |
[24] | Ekberg C, Petranikova M (2015) Lithium batteries recycling, In: Chagnes A, Światowska J, Lithium Process Chemistry, Amsterdam: Elsevier Inc, 233–267. https://doi.org/10.1016/B978-0-12-801417-2.00007-4 |
[25] | 2019 Map and List of North America's Largest MRFs (2022). Available from: https://www.zeemaps.com/mobile?group=3528074. |
[26] | Saha AK, Jin H (2023) Optimizing reverse logistics supply Chain network for sustainable value recovery from Li-ion batteriesin the United States. https://doi.org/10.2139/ssrn.4411923 |
[27] | Electricity price by state (2023). Available from: https://www.eia.gov/electricity/monthly/epm_table_grapher.php?t=epmt_5_6_a. |
[28] | Google Maps (2022). |
[29] | Mann MK (2019) Battery recycling supply chain analysis. National Renewable Energy Lab.(NREL), Golden, CO (United States). Available from: https://www.osti.gov/biblio/1559786. |
[30] | United States Environment Protection Agency (2022). Available from: https://www.epa.gov/planandbudget/strategicplan. |
[31] | Dai Q, Spangenberger J, Ahmed S, et al. (2019) EverBatt: A closed-loop battery recycling cost and environmental impacts model. Argonne National Laboratory (ANL), Argonne, IL (United States), 1–88. https://doi.org/10.2172/1530874 |
[32] | U.S. Geological Survey (2023) Mineral commodity summaries 2023. Available from: https://www.usgs.gov/publications/mineral-commodity-summaries-2023. |
[33] | Wang S, Yu J (2021) A comparative life cycle assessment on lithium-ion battery: Case study on electric vehicle battery in China considering battery evolution. Waste Manage Res 39: 156–164. https://doi.org/10.1177/0734242X2096 doi: 10.1177/0734242X2096 |
[34] | Alipanah M, Jin H, Zhou Q, et al. (2023) Sustainable bioleaching of lithium-ion batteries for critical materials recovery: Process optimization through design of experiments and thermodynamic modeling. Resour Conserv Recy 199: 107293. https://doi.org/10.1016/j.resconrec.2023.107293 doi: 10.1016/j.resconrec.2023.107293 |