Research article

Coal gasification by indirect heating in a single moving bed reactor: Process development & simulation

  • Received: 14 April 2015 Accepted: 14 October 2015 Published: 19 October 2015
  • In this work, the development and simulation of a new coal gasification process with indirect heat supply is performed. In this way, the need of pure oxygen production as in a conventional gasification process is avoided. The feasibility and energetic self-sufficiency of the proposed processes are addressed. To avoid the need of Air Separation Unit, the heat required by gasification reactions is supplied by the combustion flue gases, and transferred to the reacting mixture through a bayonet heat exchanger installed inside the gasifier. Two alternatives for the flue gas generation have been investigated and compared. The proposed processes are modeled using chemical kinetics validated on experimental gasification data by means of a standard process simulator (Aspen PlusTM), integrated with a spreadsheet for the modeling of a special type of heat exchanger. Simulation results are presented and discussed for proposed integrated process schemes. It is shown that they do not need external energy supply and ensure overall efficiencies comparable to conventional processes while producing syngas with lower content of carbon dioxide.

    Citation: Junaid Akhlas, Silvia Baesso, Alberto Bertucco, Fabio Ruggeri. Coal gasification by indirect heating in a single moving bed reactor: Process development & simulation[J]. AIMS Energy, 2015, 3(4): 635-665. doi: 10.3934/energy.2015.4.635

    Related Papers:

  • In this work, the development and simulation of a new coal gasification process with indirect heat supply is performed. In this way, the need of pure oxygen production as in a conventional gasification process is avoided. The feasibility and energetic self-sufficiency of the proposed processes are addressed. To avoid the need of Air Separation Unit, the heat required by gasification reactions is supplied by the combustion flue gases, and transferred to the reacting mixture through a bayonet heat exchanger installed inside the gasifier. Two alternatives for the flue gas generation have been investigated and compared. The proposed processes are modeled using chemical kinetics validated on experimental gasification data by means of a standard process simulator (Aspen PlusTM), integrated with a spreadsheet for the modeling of a special type of heat exchanger. Simulation results are presented and discussed for proposed integrated process schemes. It is shown that they do not need external energy supply and ensure overall efficiencies comparable to conventional processes while producing syngas with lower content of carbon dioxide.


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    [1] Lucquiaud M, Gibbins J (2011) On the integration of CO2 capture with coal-fired power plants: a methodology to assess and optimise solvent-based post-combustion capture systems. Chem Eng Res Des 89: 1553-1571. doi: 10.1016/j.cherd.2011.03.003
    [2] EU Commission (2006) Commission communication on sustainable power generation from fossil fuels: aiming from near zero emissions from coal after 2020. Summary of the impact assessment. SEC 1723.
    [3] Engelbrecht AD, North BC, Oboirien BO (2010) Making the most of South Africa's low-quality coal: Converting high-ash coal to fuel gas using bubbling fluidised bed gasifiers. In: CSIR, Science Real and Relevant Conference, Pretoria (South Africa), EN06-PA-F.
    [4] Sudiro M, Pellizzaro M, Bezzo F, et al. (2010b) Simulated moving bed technology applied to coal gasification. Chem Eng Res Des 88: 465-475.
    [5] Wen CY, Desai PR, Lin CY (1975) Factors Affecting the Thermal Efficiency of a Gasification Process. Chem Soc Div Fuel Chem Prepr 20: 219-226.
    [6] Majoumerd MM, Raas H, De S, et al. (2014) Estimation of performance variation of future generation IGCC with coal quality and gasification process—Simulation results of EU H2-IGCC project. Appl Energy 113: 452-462. doi: 10.1016/j.apenergy.2013.07.051
    [7] Higman C, Van der Burgt M (2008) Gasification. Gulf Professional Publishing, Elsevier Science (USA).
    [8] Bayarsaikhan B, Sonoyama N, Hosokai S, et al. (2006) Inhibition of steam gasification of char by volatiles in a fluidized bed under continuous feeding of a brown coal. Fuel 85: 340-349. doi: 10.1016/j.fuel.2005.06.001
    [9] Wen CY, Chen H, Onozaki M (1982) User's Manual for Computer Simulation and Design of the Moving Bed Coal Gasifier. DOE/MC/16474-1390.
    [10] Sudiro M, Bertucco A, Ruggeri F, et al. (2008) Improving Process Performances in Coal Gasification for Power and Synfuel Production. Energy Fuels 22: 3894-3901.
    [11] Sudiro M, Zanella C, Bertucco A, et al. (2010a) Dual-Bed Gasification of Petcoke: Model Development and Validation. Energy Fuels 24: 1213-1221.
    [12] Zhang Y, Wang Y, Cai L, et al. (2013) Dual bed pyrolysis gasification of coal: Process analysis and pilot test. Fuel 112: 624-634.
    [13] Arthur CJ, Munir MT, Young BR, et al. (2014) Process simulation of the transport gasifier. Fuel 115: 479-489.
    [14] Feng X, He C, Chu KH (2013) Process modeling and thermodynamic analysis of Lurgi fixed-bed coal gasifier in an SNG plant. Appl Energy 111: 742-757. doi: 10.1016/j.apenergy.2013.05.045
    [15] Kawabata M, Kurata O, Iki N, et al. (2012) Advanced integrated gasification combined cycle (A-IGCC) by exergy recuperation—technical challenges for future generations. J Power Tech 92: 90-100.
    [16] Duan W, Yu Q, Xie H, et al. (2014) Thermodynamic analysis of hydrogen-rich gas generation from coal/steam gasification using blast furnace slag as heat carrier. Int J Hydrogen Energy 39: 11611-11619. doi: 10.1016/j.ijhydene.2014.05.125
    [17] O'Doherty T, Jolly AJ, Bates CJ (2001) Analysis of a bayonet tube heat exchanger. Appl Therm Eng 21: 1-18. doi: 10.1016/S1359-4311(99)00063-0
    [18] McKetta JJ (1992) Heat Transfer Design Methods. New York (USA): M. Dekker.
    [19] Hobbs ML, Radulovic PT, Smoot LD (1992) Modeling fixed-bed coal gasifiers. AIChE J 38: 681-702.
    [20] Larson ED, Jin H, Celik F (2004) Production of Electricity and/or Fuels from Biomass by Thermochemical Conversion. In: RBAEF Meeting, Washington, D.C. (USA).
    [21] Luberti M, Friedrich D, Ozcan DC, et al. (2014) Cogeneration of ultrapure hydrogen and power at an advanced integrated gasification combined cycle with pre-combustion capture. In: The 12th IChemE European Gasification Conference: New Horizons in Gasification, Rotterdam (Netherlands).
    [22] Benson SA, Sondreal EA, Hurley JP (1995) Status of coal ash behavior research. Fuel Process Technol 44: 1-12.
    [23] Aspen Plus (2012) Model for Moving Bed Coal Gasifier, v8.0. Berlington, USA.
    [24] Suuberg EM, Peters WA, Howard JB (1978) Product composition and kinetics of lignite pyrolysis. Ind Eng Chem Process Des Dev 17: 37-46.
    [25] Rinard IH, Benjamin BW (1985) Great plains ASPEN model development: gasifier model. Literature Review and Model Specification. DOE/MC/19163-1782.
    [26] Wen CY, Chaung TZ (1979) Entrainment coal gasification modelling. Ind Eng Chem Process Des Dev 18: 684-695. doi: 10.1021/i260072a020
    [27] Bussman W, Baukal C, French K. Variable Test Furnace Cooling. 2005 Summer Heat Transfer Conference, San Francisco (USA). HT2005-72012.
    [28] Foster Wheeler Italiana S.p.a., 2013, Personal communication.
    [29] Institute of Gas Technology (1976) Coal Conversion Systems Technical Data Book, Section PMa. 44.1.
    [30] Zheng L, Furinsky E (2005) Comparison of Shell, Texaco, BGL and KRW gasifiers as part of IGCC plant computer simulations. Energ Convers Manage 46: 1767-1779. doi: 10.1016/j.enconman.2004.09.004
    [31] Kunii D, Levenspiel O (1991) Fluidization engineering. 2nd edition. Boston, USA: Butterworth-Heinemann.
    [32] Cen KF, Ni MJ, Luo ZY, et al. (1998) Theory, design and operation of circulating fluidized bed boilers. Chinese Electric Power Press, Beijing (China).
    [33] Dittus FW, Boelter LMK (1930) Heat Transfer in Turbulent Pipe and Channel Flow. Publications on Engineering, University of California, Berkeley 2: 443-461.
    [34] Incropera FP; Dewitt DP (2001) Fundamentals of Heat and Mass Transfer. New York, USA: Wiley.
    [35] Wiberg R, Lior N (2005) Heat transfer from a cylinder in axial turbulent flows. Int J Heat Mass Transfer 48: 1505-1517. doi: 10.1016/j.ijheatmasstransfer.2004.10.015
    [36] Munro RG (1997) Material Properties of a Sintered α-SiC. Ceramics Division, National Institute of Standards and Technology, Gaithersburg, Maryland 20899, USA.
    [37] Kubota Metal Corporation. Available from: http://www.kubotametal.com/alloys/heat_resistant/ hk-40.pdf (accessed 26-Jun-2014).
    [38] NiPERA (Nickel Producers Environmental Research Association) (1974) Cast heat-resistant alloys. Available from: http://www.nipera.org/~/Media/Files/TechnicalLiterature/CastHeat_ ResistantAlloys_ 1196_.pdf (accessed 28-Nov-2014).
    [39] Emissivity of Common Materials. Available from: http://www.omega.com/literature/transactions/volume1/emissivitya.html (accessed 26-Jun-2014).
    [40] http://www.sentrotech.com/shop/silicon-carbide-tubes-6978 (accessed 26-Jun-2014).
    [41] Emissivity of Common Materials. Available from: http://www.omega.com/literature/transactions/volume1/emissivityb.html (accessed 26-Jun-2014).
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